Molecular artificial photosynthesis

Serena Berardi, Samuel Drouet, Laia Francàs, Carolina Gimbert-Suriñach, Miguel Guttentag, Craig Richmond, Thibaut Stoll, Antoni Llobet

Research output: Contribution to journalReview articleResearchpeer-review

484 Citations (Scopus)

Abstract

© the Partner Organisations 2014. The replacement of fossil fuels by a clean and renewable energy source is one of the most urgent and challenging issues our society is facing today, which is why intense research has been devoted to this topic recently. Nature has been using sunlight as the primary energy input to oxidise water and generate carbohydrates (solar fuel) for over a billion years. Inspired, but not constrained, by nature, artificial systems can be designed to capture light and oxidise water and reduce protons or other organic compounds to generate useful chemical fuels. This tutorial review covers the primary topics that need to be understood and mastered in order to come up with practical solutions for the generation of solar fuels. These topics are: the fundamentals of light capturing and conversion, water oxidation catalysis, proton and CO2 reduction catalysis and the combination of all of these for the construction of complete cells for the generation of solar fuels.
Original languageEnglish
Pages (from-to)7501-7519
JournalChemical Society Reviews
Volume43
Issue number22
DOIs
Publication statusPublished - 1 Jan 2014

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