Misfit Dislocation Guided Topographic and Conduction Patterning in Complex Oxide Epitaxial Thin Films

Felip Sandiumenge, Núria Bagués, José Santiso, Markos Paradinas, Alberto Pomar, Zorica Konstantinovic, Carmen Ocal, Lluís Balcells, Marie Jo Casanove, Benjamín Martínez

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    11 Citations (Scopus)

    Abstract

    © 2016 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim Interfacial dissimilarity has emerged in recent years as the cornerstone of emergent interfacial phenomena, while enabling the control of electrical transport and magnetic behavior of complex oxide epitaxial films. As a step further toward the lateral miniaturization of functional nanostructures, this work uncovers the role of misfit dislocations in creating periodic surface strain patterns that can be efficiently used to control the spatial modulation of mass transport phenomena and bandwidth-dependent properties on a ≈20 nm length scale. The spontaneous formation of surface strain-relief patterns in La0.7Sr0.3MnO3/LaAlO3 films results in lateral periodic modulations of the surface chemical potential and tetragonal distortion, controlling the spatial distribution of preferential nucleation sites and the bandwidth of the epilayer, respectively. These results provide insights into the spontaneous formation of strain-driven ordered surface patterns, topographic and functional, during the growth of complex oxide heterostructures on lengths scales far below the limits achievable through top-down approaches.
    Original languageEnglish
    Article number1600106
    JournalAdvanced Materials Interfaces
    Volume3
    Issue number14
    DOIs
    Publication statusPublished - 22 Jul 2016

    Keywords

    • complex oxides
    • misfit dislocations
    • strain
    • surface current
    • surface patterning

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