Metallic nanoparticles enhanced the spontaneous emission of semiconductor nanocrystals embedded in nanoimprinted photonic crystals

V. Reboud; G. Lévêque; M. Striccoli; T. Placido; A. Panniello; M. L. Curri; J. A. Alducin; T. Kehoe; N. Kehagias; D. Mecerreyes; S. B. Newcomb; D. Iacopino; G. Redmond; C. M.Sotomayor Torres

doi:10.1039/c2nr32134c

Metallic nanoparticles enhanced the spontaneous emission of semiconductor nanocrystals embedded in nanoimprinted photonic crystals

V. Reboud, G. Lévêque, M. Striccoli, T. Placido, A. Panniello, M. L. Curri, J. A. Alducin, T. Kehoe, N. Kehagias, D. Mecerreyes, S. B. Newcomb, D. Iacopino, G. Redmond, C. M.Sotomayor Torres

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12 Citations (Scopus)

Abstract

We report on a method to enhance the light-emission efficiency of printable thin films of a polymer doped with luminescent (CdSe)ZnS nanocrystals via metallic nanoparticles and nanoimprinted photonic crystals. We experimentally show a strong fluorescence enhancement of nanocrystals by coupling exciton-plasmon with the localized surface plasmon of metallic nanoparticles. The emitted light is efficiently diffracted by photonic crystals structures directly imprinted in the nanocomposite polymer. By combining the field susceptibility technique with optical Bloch equations, we examine the interaction of the quantum and plasmonic entities at small distances. © 2013 The Royal Society of Chemistry.

Original language	English
Pages (from-to)	239-245
Journal	Nanoscale
Volume	5
Issue number	1
DOIs	https://doi.org/10.1039/c2nr32134c
Publication status	Published - 7 Jan 2013

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Reboud, V., Lévêque, G., Striccoli, M., Placido, T., Panniello, A., Curri, M. L., Alducin, J. A., Kehoe, T., Kehagias, N., Mecerreyes, D., Newcomb, S. B., Iacopino, D., Redmond, G., & Torres, C. M. S. (2013). Metallic nanoparticles enhanced the spontaneous emission of semiconductor nanocrystals embedded in nanoimprinted photonic crystals. Nanoscale, 5(1), 239-245. https://doi.org/10.1039/c2nr32134c

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title = "Metallic nanoparticles enhanced the spontaneous emission of semiconductor nanocrystals embedded in nanoimprinted photonic crystals",

abstract = "We report on a method to enhance the light-emission efficiency of printable thin films of a polymer doped with luminescent (CdSe)ZnS nanocrystals via metallic nanoparticles and nanoimprinted photonic crystals. We experimentally show a strong fluorescence enhancement of nanocrystals by coupling exciton-plasmon with the localized surface plasmon of metallic nanoparticles. The emitted light is efficiently diffracted by photonic crystals structures directly imprinted in the nanocomposite polymer. By combining the field susceptibility technique with optical Bloch equations, we examine the interaction of the quantum and plasmonic entities at small distances. {\textcopyright} 2013 The Royal Society of Chemistry.",

author = "V. Reboud and G. L{\'e}v{\^e}que and M. Striccoli and T. Placido and A. Panniello and Curri, {M. L.} and Alducin, {J. A.} and T. Kehoe and N. Kehagias and D. Mecerreyes and Newcomb, {S. B.} and D. Iacopino and G. Redmond and Torres, {C. M.Sotomayor}",

year = "2013",

month = jan,

day = "7",

doi = "10.1039/c2nr32134c",

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journal = "Nanoscale",

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Reboud, V, Lévêque, G, Striccoli, M, Placido, T, Panniello, A, Curri, ML, Alducin, JA, Kehoe, T, Kehagias, N, Mecerreyes, D, Newcomb, SB, Iacopino, D, Redmond, G & Torres, CMS 2013, 'Metallic nanoparticles enhanced the spontaneous emission of semiconductor nanocrystals embedded in nanoimprinted photonic crystals', Nanoscale, vol. 5, no. 1, pp. 239-245. https://doi.org/10.1039/c2nr32134c

TY - JOUR

T1 - Metallic nanoparticles enhanced the spontaneous emission of semiconductor nanocrystals embedded in nanoimprinted photonic crystals

AU - Reboud, V.

AU - Lévêque, G.

AU - Striccoli, M.

AU - Placido, T.

AU - Panniello, A.

AU - Curri, M. L.

AU - Alducin, J. A.

AU - Kehoe, T.

AU - Kehagias, N.

AU - Mecerreyes, D.

AU - Newcomb, S. B.

AU - Iacopino, D.

AU - Redmond, G.

AU - Torres, C. M.Sotomayor

PY - 2013/1/7

Y1 - 2013/1/7

N2 - We report on a method to enhance the light-emission efficiency of printable thin films of a polymer doped with luminescent (CdSe)ZnS nanocrystals via metallic nanoparticles and nanoimprinted photonic crystals. We experimentally show a strong fluorescence enhancement of nanocrystals by coupling exciton-plasmon with the localized surface plasmon of metallic nanoparticles. The emitted light is efficiently diffracted by photonic crystals structures directly imprinted in the nanocomposite polymer. By combining the field susceptibility technique with optical Bloch equations, we examine the interaction of the quantum and plasmonic entities at small distances. © 2013 The Royal Society of Chemistry.

AB - We report on a method to enhance the light-emission efficiency of printable thin films of a polymer doped with luminescent (CdSe)ZnS nanocrystals via metallic nanoparticles and nanoimprinted photonic crystals. We experimentally show a strong fluorescence enhancement of nanocrystals by coupling exciton-plasmon with the localized surface plasmon of metallic nanoparticles. The emitted light is efficiently diffracted by photonic crystals structures directly imprinted in the nanocomposite polymer. By combining the field susceptibility technique with optical Bloch equations, we examine the interaction of the quantum and plasmonic entities at small distances. © 2013 The Royal Society of Chemistry.

U2 - 10.1039/c2nr32134c

DO - 10.1039/c2nr32134c

M3 - Article

SN - 2040-3364

VL - 5

SP - 239

EP - 245

JO - Nanoscale

JF - Nanoscale

IS - 1

ER -

Metallic nanoparticles enhanced the spontaneous emission of semiconductor nanocrystals embedded in nanoimprinted photonic crystals

Abstract

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