Incommensurate magnetic structures of multiferroic MnWO<inf>4</inf> studied within the superspace formalism

I. Urcelay-Olabarria, J. M. Perez-Mato, J. L. Ribeiro, J. L. García-Muñoz, E. Ressouche, V. Skumryev, A. A. Mukhin

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Abstract

The magnetic structures of the incommensurate phases of the prototypic multiferroic MnWO4 are analyzed using superspace symmetry formalism. This approach shows in a very simple way the relation between the magnetic symmetry of the incommensurate phases and any tensorial property, such as ferroelectricity. The magnetic structures have been redetermined by single-crystal neutron diffraction experiments, which revealed fine details of the AF3 and AF2 magnetic structures. The spin modulations of the two manganese ions of the basic unit cell are symmetry-related in the paraelectric incommensurate-magnetic structure (AF3) - they are not forced to be collinear but they must have opposite chirality - while in the multiferroic phase (AF2) they become symmetry independent. It is due to this symmetry break that the electric polarization arises along the b axis. © 2013 American Physical Society.
Original languageEnglish
Article number014419
JournalPhysical Review B - Condensed Matter and Materials Physics
Volume87
Issue number1
DOIs
Publication statusPublished - 15 Jan 2013

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