Single-Crystal-to-Single-Crystal Postsynthetic Modification of a Metal-Organic Framework via Ozonolysis

Jorge Albalad, Heng Xu, Felipe Gándara, Mohamed Haouas, Charlotte Martineau-Corcos, Rubén Mas-Ballesté, Sarah A. Barnett, Judith Juanhuix, Inhar Imaz, Daniel Maspoch

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    Resum

    © 2018 American Chemical Society. We describe solid-gas phase, single-crystal-to-single-crystal, postsynthetic modifications of a metal-organic framework (MOF). Using ozone, we quantitatively transformed the olefin groups of a UiO-66-type MOF into 1,2,4-trioxolane rings, which we then selectively converted into either aldehydes or carboxylic acids.
    Idioma originalAnglès
    Pàgines (de-a)2028-2031
    RevistaJournal of the American Chemical Society
    Volum140
    Número6
    DOIs
    Estat de la publicacióPublicada - 14 de febr. 2018

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