Coassembly of Complementary Polyhedral Metal-Organic Framework Particles into Binary Ordered Superstructures

Lingxin Meng, Javier Fonseca, Roberto Sánchez-Naya, Amir Mohammad Ghadiri, Inhar Imaz, Daniel Maspoch Comamala

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Resum

Here we report the formation of a 3D NaCl-type binary porous superstructure via coassembly of two colloidal polyhedral metal-organic framework (MOF) particles having complementary sizes, shapes, and charges. We employed a polymeric-attenuated Coulombic self-assembly approach, which also facilitated the coassembly of these MOF particles with spherical polystyrene particles to form 2D binary superstructures. Our results pave the way for using MOFs to create sophisticated superstructures comprising particles of various sizes, shapes, porosities, and chemical compositions.
Idioma originalAnglès
Pàgines (de-a)21225-21230
Nombre de pàgines6
RevistaJournal of the American Chemical Society
Volum146
Número31
DOIs
Estat de la publicacióPublicada - 26 de jul. 2024

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